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            Abstract Unexpected, yet useful functionalities emerge when two or more materials merge coherently. Artificial oxide superlattices realize atomic and crystal structures that are not available in nature, thus providing controllable correlated quantum phenomena. This review focuses on 4d and 5d perovskite oxide superlattices, in which the spin–orbit coupling plays a significant role compared with conventional 3d oxide superlattices. Modulations in crystal structures with octahedral distortion, phonon engineering, electronic structures, spin orderings, and dimensionality control are discussed for 4d oxide superlattices. Atomic and magnetic structures,Jeff= 1/2 pseudospin and charge fluctuations, and the integration of topology and correlation are discussed for 5d oxide superlattices. This review provides insights into how correlated quantum phenomena arise from the deliberate design of superlattice structures that give birth to novel functionalities.more » « less
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            Jeong, Seung Gyo; Kim, Jiwoong; Seo, Ambrose; Park, Sungkyun; Jeong, Hu Young; Kim, Young-Min; Lauter, Valeria; Egami, Takeshi; Han, Jung Hoon; Choi, Woo Seok (, Science Advances)Chiral phonons and their strong coupling to spins reveal unconventional interlayer exchange interaction and resultant spin state.more » « less
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            Ok, Jong Mok; Mohanta, Narayan; Zhang, Jie; Yoon, Sangmoon; Okamoto, Satoshi; Choi, Eun Sang; Zhou, Hua; Briggeman, Megan; Irvin, Patrick; Lupini, Andrew R.; et al (, Science Advances)Quantum materials (QMs) with strong correlation and nontrivial topology are indispensable to next-generation information and computing technologies. Exploitation of topological band structure is an ideal starting point to realize correlated topological QMs. Here, we report that strain-induced symmetry modification in correlated oxide SrNbO 3 thin films creates an emerging topological band structure. Dirac electrons in strained SrNbO 3 films reveal ultrahigh mobility (μ max ≈ 100,000 cm 2 /Vs), exceptionally small effective mass ( m * ~ 0.04 m e ), and nonzero Berry phase. Strained SrNbO 3 films reach the extreme quantum limit, exhibiting a sign of fractional occupation of Landau levels and giant mass enhancement. Our results suggest that symmetry-modified SrNbO 3 is a rare example of correlated oxide Dirac semimetals, in which strong correlation of Dirac electrons leads to the realization of a novel correlated topological QM.more » « less
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